文献类型：期刊文献

英文题名：Biochar-based materials and their applications in removal of organic contaminants from wastewater: state-of-the-art review

作者：Huang, Qiang[1,2];Song, Shuang[1];Chen, Zhe[1];Hu, Baowei[2];Chen, Jianrong[3];Wang, Xiangke[1]

机构：[1]North China Elect Power Univ, Coll Environm Sci & Engn, MOE Key Lab Resources & Environm Syst Optimizat, Beijing 102206, Peoples R China;[2]Shaoxing Univ, Sch Life Sci, Huancheng West Rd 508, Shaoxing 312000, Peoples R China;[3]Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Zhejiang, Peoples R China

年份：2019

卷号：1

期号：1

起止页码：45

外文期刊名：BIOCHAR

收录：SCI-EXPANDED(收录号：WOS:000646950300004)、、WOS

基金：The authors thank the financial support from the National Key Research and Development Program of China (2017YFA0207002), the National Natural Science Foundation of China (21836001, 21607042) and the Fundamental Research Funds for the Central Universities (2018ZD11, 2018MS114).

语种：英文

外文关键词：Biochar-based materials; Water purification; Organic contaminants; Catalytic degradation; Adsorption

外文摘要：As a class of famous carbon materials, biochars (BCs) and their derivative materials with excellent physicochemical properties and diversified functionalities present great potential in wastewater treatment fields. This review focuses on the latest development in reported biochar-based materials as superior adsorbents or catalysts for removing harmful organic contaminants from wastewater. The construction and properties of biochar-based materials are briefly introduced at the beginning. As one of the major factors affecting the properties of BCs, the wide diversity of feedstocks, such as agricultural and forest residues, industrial by-products as well as municipal wastes, endows BCs different chemical compositions and structures. Woody and herbaceous BCs usually have higher carbon contents, larger surface areas and strong aromaticity, which is in favor of the organic contaminant removal. Driven by the desire of more cost-effective materials, several types of biochar-based hybrid materials, such as magnetic BC composites (MBC), nanometal/nanometallic oxides/hydroxide BC composites and layered nanomaterial-coated BCs, as well as physically/chemically activated BCs, have also been developed. With the help of foreign materials, these types of hybrid BCs have excellent capacities to remove a wide range of organic contaminants, including organic dyestuff, phenols and chemical intermediates, as well as pharmaceutically active compounds, from aquatic solutions. Depending on the different types of biochar-based materials, organic contaminants can be removed by different mechanisms, such as physical adsorption, electrostatic interaction, pi-pi interaction and Fenton process, as well as photocatalytic degradation. In summary, the low cost, tunable surface chemistry and excellent physical-chemical properties of BCs allow it to be a potential material in organic contaminant removal. The combination of BCs with foreign materials endows BCs more functionalities and broader development opportunities. Considering the urgent demand of practical wastewater treatment, we hope more researches will focus on the applications and commercialization of biochar-based materials.