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Applications of water-stable metal-organic frameworks in the removal of water pollutants: A review  ( SCI-EXPANDED收录 EI收录)   被引量:321

文献类型:期刊文献

英文题名:Applications of water-stable metal-organic frameworks in the removal of water pollutants: A review

作者:Zhang, Shu[1];Wang, Jiaqi[1];Zhang, Yue[1];Ma, Junzhou[1];Huang, Lintianyang[1];Yu, Shujun[2];Chen, Lan[1];Song, Gang[3];Qiu, Muqing[4];Wang, Xiangxue[1,5]

机构:[1]North China Elect Power Univ, Dept Environm Sci & Engn, Hebei Key Lab Power Plant Flue Gas Multipollutant, Baoding 071003, Peoples R China;[2]North China Elect Power Univ, Coll Environm Sci & Engn, MOE Key Lab Resources & Environm Syst Optimizat, Beijing 102206, Peoples R China;[3]Guangzhou Univ, Sch Environm Sci & Engn, Guangdong Prov Key Lab Radionuclides Pollut Contr, Guangzhou 510006, Peoples R China;[4]Shaoxing Univ, Sch Life Sci, Shaoxing 312000, Peoples R China;[5]Southwest Univ Sci & Technol, Fdn Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Sichuan, Peoples R China

年份:2021

卷号:291

外文期刊名:ENVIRONMENTAL POLLUTION

收录:SCI-EXPANDED(收录号:WOS:000696628800005)、、EI(收录号:20213710900476)、Scopus(收录号:2-s2.0-85114780443)、WOS

基金:This work was supported by National Key Research and Development Program of China (2017YFA0207002), the National Natural Science Foundation of China (21906052, U2067215), the Research Fund Program of Guangdong Provincial Key Laboratory of Radionuclides Pollution Control and Resources (2017B030314182), the Open Foundation of Fundamental Science on Nuclear Waste and Environmental Security Laboratory (17kfhk01).

语种:英文

外文关键词:Water-stable MOFs; UiO; MIL; ZIF; Environmental remediation

外文摘要:Because the pollutants produced by human activities have destroyed the ecological balance of natural water environment, and caused severe impact on human life safety and environmental security. Hence the task of water environment restoration is imminent. Metal-organic frameworks (MOFs), structured from organic ligands and inorganic metal ions, are notable for their outstanding crystallinity, diverse structures, large surface areas, adsorption performance, and excellent component tunability. The water stability of MOFs is a key requisite for their possible actual applications in separation, catalysis, adsorption, and other water environment remediation areas because it is necessary to safeguard the integrity of the material structure during utilization. In this article, we comprehensively review state-of-the-art research progress on the promising potential of MOFs as excellent nanomaterials to remove contaminants from the water environment. Firstly, the fundamental characteristics and preparation methods of several typical water-stable MOFs include UiO, MIL, and ZIF are introduced. Then, the removal property and mechanism of heavy metal ions, radionuclide contaminants, drugs, and organic dyes by different MOFs were compared. Finally, the application prospect of MOFs in pollutant remediation prospected. In this review, the synthesis methods and application in water pollutant removal are explored, which provide ways toward the effective use of water-stable MOFs in materials design and environmental remediation.

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