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Low-temperature plasma induced phosphate groups onto coffee residue-derived porous carbon for efficient U(VI) extraction  ( SCI-EXPANDED收录 EI收录)   被引量:40

文献类型:期刊文献

英文题名:Low-temperature plasma induced phosphate groups onto coffee residue-derived porous carbon for efficient U(VI) extraction

作者:Chen, Zhongshan[1,2];He, Xuan[2];Li, Qian[2];Yang, Hui[2];Liu, Yang[2];Wu, Lining[3];Liu, Zhixin[1];Hu, Baowei[1];Wang, Xiangke[1,2]

机构:[1]Shaoxing Univ, Sch Life Sci, Shaoxing 312000, Peoples R China;[2]North China Elect Power Univ, Coll Environm Sci & Engn, Beijing 102206, Peoples R China;[3]North China Elect Power Univ, Sch Energy Power & Mech Engn, Beijing 102206, Peoples R China

年份:2022

卷号:122

起止页码:1

外文期刊名:JOURNAL OF ENVIRONMENTAL SCIENCES

收录:SCI-EXPANDED(收录号:WOS:000798823500001)、、EI(收录号:20220511569148)、Scopus(收录号:2-s2.0-85123676613)、WOS

基金:This work was supported by the National Key Research and Development Program of China (Nos. 2018YFC1900105; 2016YFA0203200; 2017YFA0207002), the Beijing Outstanding Young Scientist Program and the Fundamental Research Funds for the Central Universities (No. 2019MS044).

语种:英文

外文关键词:U(VI); Coffee residue; Porous carbon; Low-temperature plasma; modification

外文摘要:For the continuous utilization of nuclear energy and efficient control of radioactive pollution, low-cost materials with high efficient U(VI) removal are of great importance. In this study, low temperature plasma method was applied for the successful modification of Ophosphorylethanolamine (O-PEA) on the porous carbon materials. The produced materials (Cafe/O-PEA) could adsorb U(VI) efficiently with the maximum sorption capacity of 648.54 mg/g at 1 hr, T = 298K, and pH = 6.0, much higher than those of most carbon-based composites. U(VI) sorption was mainly controlled by strong surface complexation. From FTIR, SEMEDS and XPS analyses, the sorption of U(VI) was related to the complexation with -NH 2 , phosphate and -OH groups on Cafe/O-PEA. The low temperature plasma method was an efficient, environmentally friendly and low-cost method for surface modification of materials for the effective enrichment of U(VI) from aqueous solutions. ?? 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

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